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Yuan, Wei; Yan, Zi-Jie; Yi, Hemian; Wang, Zihao; Paolini, Stephen; Zhao, Yi-Fan; Zhou, Lingjie; Wang, Annie G; Wang, Ke; Prokscha, Thomas; et al (, Nano Letters)
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Wang, Fei; Zhao, Yi-Fan; Yan, Zi-Jie; Zhuo, Deyi; Yi, Hemian; Yuan, Wei; Zhou, Lingjie; Zhao, Weiwei; Chan, Moses H.; Chang, Cui-Zu (, Nano Letters)To date, the quantum anomalous Hall effect has been realized in chromium (Cr)- and/or vanadium(V)-doped topological insulator (Bi,Sb)2Te3 thin films. In this work, we use molecular beam epitaxy to synthesize both V- and Cr-doped Bi2Te3 thin films with controlled dopant concentration. By performing magneto-transport measurements, we find that both systems show an unusual yet similar ferromagnetic response with respect to magnetic dopant concentration; specifically the Curie temperature does not increase monotonically but shows a local maximum at a critical dopant concentration. We attribute this unusual ferromagnetic response observed in Cr/V-doped Bi2Te3 thin films to the dopant-concentration-induced magnetic exchange interaction, which displays evolution from van Vleck-type ferromagnetism in a nontrivial magnetic topological insulator to Ruderman–Kittel–Kasuya–Yosida (RKKY)-type ferromagnetism in a trivial diluted magnetic semiconductor. Our work provides insights into the ferromagnetic properties of magnetically doped topological insulator thin films and facilitates the pursuit of high-temperature quantum anomalous Hall effect.more » « less
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Takeshige, Yuusuke; Matsuo, Sadashige; Deacon, Russell S.; Ueda, Kento; Sato, Yosuke; Zhao, Yi-Fan; Zhou, Lingjie; Chang, Cui-Zu; Ishibashi, Koji; Tarucha, Seigo (, Physical Review B)
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